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Compared to TePP and you will pentaphenylpyrrole (PPP), each other TPM and you can TPM-Cl demonstrated prolonged emission wavelengths. Thanks to the similar chemicals formations, this is simply not plausible so you can feature the key Stokes shift to differences in the ability pit involving the reduced singlet excited county (S1) and you may soil county (S0). I thus propose that the new red emission represents a decreased triplet thrilled condition (T1), that is less than S1. dos, the spot where the contours are exactly the same on their constant-state emission spectra, sharing the brand new a lot of time lifestyle services out of both TPM and you will TPM-Cl. The new lifetimes of the TPM and you will TPM-Cl crystalline powders try 20.1 and 8.9 μs, correspondingly (Fig. S3 and you will Desk S1).
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Chongqing Wulong Karst Area, Wulong Karst Surroundings
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